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A series of boron, aluminum, gallium, and indium chelates containing the underexplored bis(phenolate) aza-dipyrromethene (aza-DIPY) core were prepared. These compounds were found to possess near-infrared absorption and emission profiles in the 710 to 770 nm domain and exhibit quantum yield values up to 14%. X-ray diffraction analysis revealed that heavier group 13 bis(phenolate) aza-DIPY chelates possessed octahedral geometries with either THF or pyridine groups occupying the axial positions as opposed to the tetrahedral geometry of the boron chelate.more » « less
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Neal, Martin J. ; Hejnosz, Sarah L. ; Rohde, Jeffrey J. ; Evanseck, Jeffrey D. ; Montgomery, Thomas D. ( , The Journal of Organic Chemistry)
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Hejnosz, Sarah L. ; Beres, Danielle R. ; Cocolas, Alexander H. ; Neal, Martin J. ; Musiak, Benjamin S. ; Hanna, Marianne M. B. ; Bloomfield, Aaron J. ; Montgomery, Thomas D. ( , Organic Letters)
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Montgomery, Thomas D. ; Buchbinder, Joanne Rae ; Gawalt, Ellen S. ; Iuliucci, Robbie J. ; Koch, Andrew S. ; Kotsikorou, Evangelia ; Lackey, Patrick E. ; Lim, Min Soo ; Rohde, Jeffrey Joseph ; Rupprecht, Alexander J. ; et al ( , Journal of Chemical Education)